Application of fuzzy logic to control acetylene hydrogenation reactor of olefin unit

Number of pages: 119 File Format: word File Code: 32259
Year: 2014 University Degree: Master's degree Category: Electrical Engineering
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  • Summary of Application of fuzzy logic to control acetylene hydrogenation reactor of olefin unit

    Dissertation for receiving the M.Sc degree

    Electrical Engineering - Control

    Abstract

    Given the high consumption of petrochemical products in the world today and the high potential of Iran for the development and supply of petrochemical feed, petrochemical complexes are of special importance. Therefore, one of the important reactions called acetylene hydrogenation has been investigated and controlled in one of the parent petrochemical units, i.e., the olefin unit. In this research, after reviewing the scientific reference books, scientific articles and treatises available in this field, a nonlinear acetylene hydrogenation reactor system that is being used in the petrochemical industry in the south of the country was selected and simulated using the mass and energy balance equations by the MATLAB specialized program. Then, by applying changes of a step value in reactor temperature equations, it is tried to be approximated and modeled with a suitable transformation function, with a very low error. Also, by using the step response of the approximated system, classical controllers and then fuzzy controller should be designed first, and then by showing that none of the controllers are suitable for controlling the reactor outlet temperature in the acetylene hydrogenation process, the PI_Smith fuzzy controller design is proposed with the conditions mentioned in the fourth chapter. Finally, by comparing the results of the design of different controllers for the mentioned system, it is concluded that the PI_Smith fuzzy controller can be a more suitable controller for systems with delays. rtl;">fuzzy controller design, classic controller design, acetylene hydrogenation reactor modeling

    Preface

    In the chemical industry, in order to reduce operational costs and develop new markets, there is always a special attention to improve product quality and reduce production waste. To achieve these goals, it is very necessary to use control systems. There are always many non-linear processes in the industry that cannot be controlled by classical methods, also if there are restrictions on the inputs and outputs of a process, the use of classical controllers will become much more difficult [1]. In the meantime, the fuzzy controller that has a non-linear behavior is a developing and very useful control method for non-linear processes. In addition to having a very high efficiency, it shows much more suitable behaviors in dealing with the constraints on the controlling variables, the controlled and other characteristics of the problem, and it is also suitable for systems with delays or in other words with slow dynamics.

     

    1-2- Statement of the problem

    Ethylene production [1] is one of the main indicators of growth in the petrochemical industry of any country, which is mainly used in polymer industries, especially polyethylene production. Olefin units in the petrochemical industry, where ethylene is produced, are among the mother phases. The conditions of the ethylene gas preparation process require that during the reaction, the process be free of any impurities, especially acetylene gas [2] with the symbol, ethane gas [3] with the symbol and carbon monoxide gas [4] with the symbol. For example, a small amount of acetylene impurity causes the reaction catalyst to be deactivated and thus the ethylene production process stops. Therefore, these impurities must be separated with a specific and reliable method. Acetylene is separated from ethylene by a process called hydrogenation[5] in a hydrogenation reactor. Since this process is very sensitive to temperature changes, therefore, the temperature of the hydrogenation reactor input materials should be controlled in an optimal way in order to increase the output pure ethylene gas production efficiency. Among the common problems of this reactor are its very long time delay (on the clock scale) and its nonlinear behavior.Therefore, it is expected that by considering the conditions of the acetylene hydrogenation process, by designing a suitable controller to control the temperature of the acetylene hydrogenation reactor input materials, a quality reaction will be created along with a specific production rate of the desired product of ethylene gas under optimal economic conditions [2]. rtl;">          Considering the importance of ethylene, we know that it is used as a feed for other petrochemical units, so by increasing the production efficiency of ethylene gas output from the hydrogenation reactor, it increases the quality of materials used in petrochemical industries. Therefore, by trying to increase the efficiency of ethylene production by designing suitable controllers on the acetylene hydrogenation reactor, we can overcome this goal. Also, among other things of the necessity of this research, it can be mentioned to take a positive step towards gaining the control of the important industrial processes of the country by Iranian experts using modern control sciences, such as fuzzy logic. accepted can be summarized as follows.

    As a scientific goal, it can be pointed to raise the level of knowledge of researchers and experts in the field of designing and controlling a non-linear system with delay, important and widely used in the country's industries based on fuzzy logic.

    In terms of the practical goal, it is possible to improve and upgrade conventional classical control methods used in important industrial hydrogenation processes in Petrochemicals of the country pointed out.

    Proposing a new control method, in order to reduce ethylene losses and increase the efficiency of hydrogenation reactor products, as well as considering the actual conditions in the hydrogenation reactor, in order to be closer to the actual working conditions in the country's petrochemical units.

    Designing a modern controller, which leads to reducing the response time of industrial systems Especially the delay of the acetylene hydrogenation reactor and the increase in the speed of action in removing the disturbances entering the system, without having any losses. gives, has complexity in the reactor model. This has made it impossible to identify the model of the reactor by collecting input and output data in the usual way. Therefore, as the full description of the hydrogenation reactor modeling will be discussed in the third chapter, the reactor model should be approximated by solving the mass and energy balance equations. This approximation in the model makes it impossible to always get an accurate model of the reactor for controller design. This issue in its kind is considered as a big limitation in reaching the dynamic model of the reactor and controller design. Also, among other limitations of conducting this research, we can mention the lack of access to detailed information about chemical reactors in the industry due to information protection. of the important reactions in the hydrogenation of acetylene in the main of one of petrochemical's olefin unit, too.

    In this research, after review of the scientific reference books, research papers and dissertations in the field, in the hydrogenation of acetylene nonlinear reactor systems that are used in the petrochemical industry in the south is selected by using the Mass and energy balance equations Community Planning is the MATLAB simulation. Then it is tried using a small step change in reactor temperature equation, with an appropriate conversion function, approximated by modeling error is very low. The step response approximated system, the first classic controller and fuzzy controller are designed.

  • Contents & References of Application of fuzzy logic to control acetylene hydrogenation reactor of olefin unit

    List:

    List of tables.. Y

    List of figures.. K

    Abstract.. 1

    Chapter 1 Introduction.. 2

    1-1- Preface.. 3

    1-2- Statement of the problem.. 3

    1-3- Necessity and importance of research.. 4

    1-4- The goals of the research.. 4

    1-5- Limitations in conducting the research. 5

    1-6- Research method. 6

    The second chapter of chemical reaction and chemical reactor. 8

    2-1- Introduction.. 9

    2-2- Definition of chemical reaction.. 9

    2-3- Types of chemical reactions. 10

    2-3-1- Homogeneous and non-homogeneous reactions. 10

    2-3-2- catalytic and non-catalytic reactions. 11

    2-3-3- Reversible and irreversible reactions. 11

    2-3-4- back-to-back (series) and parallel reaction. 11

    2-3-5- Endothermic and exothermic reactions. 12

    2-4- Kinetics and speed of chemical reaction. 13

    2-5- Definition of chemical reactor.. 13

    2-5-1- Reactor equation. 14

    2-6- types of chemical reactors. 14

    2-6-1- continuous, discontinuous and semi-continuous reactors. 15

    2-6-2- Fluid bed and fixed bed reactors. 17

    2-6-3- Tube reactors (plug) and tank with stirrer (CSTR). 18

    2-6-4- homogeneous and heterogeneous reactors. 20

    2-6-5- Reactors with adiabatic and non-adiabatic operation. 21

    The third chapter of acetylene hydrogenation process. 23

    3-1- Introduction.. 24

    3-2- Acetylene hydrogenation reactor. 25

    3-3- Description of the process.. 28

    3-4- History of acetylene hydrogenation reactor modeling. 32

    3-5- dynamic modeling of acetylene hydrogenation reactor. 34

    3-6- Steady state of acetylene hydrogenation process. 48

    The fourth chapter of controller design.. 52

    4-1- Introduction.. 53

    4-2- Controller definition.. 53

    4-3- Modern control.. 54

    4-3-1- Introduction to fuzzy systems. 55

    4-3-2- Belonging functions, variables and linguistic restrictions. 58

    4-3-3- Fuzzy rule base. 59

    4-3-4- Fuzzy inference engine. 59

    4-3-5- fuzzifier.. 59

    4-3-6- non-fuzzifier. 60

    4-4- Classic control.. 60

    4-5- Internal mode control (IMC). 63

    4-6- Smith predictive control.. 65

    4-7- History of acetylene hydrogenation control of olefin unit. 66

    4-8- PI controller design. 68

    4-8-1- Tyros- Luiben _ PI. 69

    4-8-2- Ziegler-Nichols _ PI. 71 4-8-3 ITAE PI. 77

    4-9- IMC controller design. 79

    4-10- Smith predictive controller design - PI. 84

    4-11- Fuzzy controller design. 87

    4-12- PI_Smith fuzzy controller design. 90

    The fifth chapter, conclusions and suggestions. 99

    5-1- Introduction.. 100

    5-2- Conclusion.. 100

    5-3- Suggestions for future research. 102

    List of references.. 104

     Abstract.. 107

     

    Source:

     

    [1] Masoud Bojari, "Predictive adaptive control of chemical reactors", Master's thesis, Sharif University of Technology, March 1382.

    [2] Hossein Hassanpour, "Catalytic Reactor Modeling of Acetylene Hydrogenation and its Comparison with Experimental Data", Master's Thesis, Sharif University of Technology, 1379.

    [3] Jenny Karpelenia, "Chemical Reactions", Perfection Learning, 2005.

    [4] Octave Lonspiel, "Chemical Reactor Design", translated by Morteza Sohrabi, Amir Kabir Industrial University Jihad, 2004. [5] Peter Atkins and Julio De Paula, “Physical Chemistry”, W.H. Freeman, 8th Edition, U.S.A, 2006. Engineers`Handbook”, Vol 1&2, New York: McGraw-Hill, 1984.

    [8] Michael K. Stenstrom and Diego Rosso, “Fundamental Of Chemical Reactor Theory”, University Of California, Los Angeles, 2003.

    [9] WWW.Controlloopfoundation.com, archive, 2013/11/25.

    [10] John Metcalfe Coulson and J.F.Richardson, "Coulson & Richardson`s Chemical Engineering",Richardson, “Coulson & Richardson`s Chemical Engineering”, Vol.3, Chemical and Biochemical Reactors & Process Control, Elsevier, 1994.

    [11] WWW.Scielo.br, archive, 2013/11/25.

    [12] Fritz Ullmann, “Ullmann`s Encyclopedia Of Industrial Chemistry”, Vol.B4, New York: John Wiley & Sons, 2011. [13] WWW.Essentialchemicalindustry.org, archive, 2013/11/25. [14] WWW. Hyperphysics.phy-astr.gsu.edu, archive, 2013/11/30. 

    [15] Farshid Nurbakhsh, "Design and Simulation of Pyrolysis Gasoline Unit in Olefin Units", Master's Thesis, Tarbiat Modares University, Spring 2018.

    [16] Michael W. Brown, Alexander Penlidis and Gerald R. Sullivan, "Control Policies for An Industrial Acetylene Hydrogenation Reactor", The Canadian Journal of Chemical Engineering, Volume 69, February 1991.

    [17] Navid Mostoufi, Ali Ghoorchiany and Rahmat Sotudeh-Gharebagh, "Hydrogenation of Acetylene: Kinetic Studies and Reactor Modeling", Vol3, International Journal of Chemical Reactor Engineering, Article A14, 2005.

    [18] R. Gobbo, R. P. Soares, M. A. Lansarin, A. R. Secchi and J. M. P. Ferreira, "Modeling, Simulation, And Optimization Of A Front-End System For Acetylene Hydrogenation Reactor", Brazilian Journal of Chemical Engineering, Vol. 21, No. 04, pp. 545 - 556, October - December 2004.

    [19] Gordon Weiss, “Modeling and Control of an Acetylene Converter”, Process Control of Elsevier, Vol.6, No.1, PP 7-15, 1996.

    [20] Stanley M.Walas, “Chemical Process Equipment”, Page 565, Butterwoth-Heinemann, 1990. [21] Luo Xionglin, Zuo Xin, Du Dianlin, "Modeling, Process Observer and Advanced Process Control of Acetylene Hydrogenation Reactor in Ethylene Complex", Proceedings of the 5th World Congress on Intelligent Control and Automation, PP 3583-3587, IEEE, June 2004. [22] Noem?´ S. Schbib, Miguel A. Garc?´a, Carlos E. G?´gola and Alberto F. Errazu, "Kinetics of Front-End Acetylene Hydrogenation in Ethylene Production", Ind. Eng. Chem. Res, 35, Page 1496-1505, 1996.

    [23] M.Szukiewics, K.Kaczmarski and R.Petrus, “Modelling of Fixed-Bed Reactor: Two Models of Industrial Reactor for Selective Hydrogenation of Acetylene”, Chemical Engineering Science, Vol.53, No.1, PP 149-155, 1998.

    [24] A.G. Abilov and M.CE KocEak, "An Optimal Control Application to An Industrial Hydrogenation Reactor", IchemE, Vol.78, Part A, May 2000.

    [25] Mehdi Rafizadeh, "Application of Mathematics in: Chemical Engineering, Polymer Engineering, Textile Engineering and Metallurgical Engineering", Publications of Amirkabir University of Technology (Tehran Polytechnic), third edition, 1384.

    [26]   Mehdi Rafizadeh, "Dynamics and control of processes with an applied approach in chemical engineering, polymer engineering and metallurgical engineering", Amirkabir University of Technology, second edition, winter 2013.

    [27] Mohammad Reza Jahid Mutlaq and Mohammad Hasan Mohadi, "The history of industrial control with a perspective on the emergence of fieldbus-based control systems", National Company of Petrochemical Industries - Iran University of Science and Technology, autumn 2013.

    [28] K.Zhou, J.C.Doyle and K.Glover, "Robust and Optimal Control", Chapter 14, 1996. [29] Li Wang, "Fuzzy Systems and Fuzzy Control", translated by Dr. Mohammad Tashnelab, Nima Safarpour and Dariush Efioni, 7th edition, Khwaja Nasiruddin Tosi University, October 2013.

    [30] W.C Dong, "Soft-sensor and Inferential Control for Acetylene Concentration of Acetylene Hydrogenation Reactor", Thesis of M.Sc, Dalian University of Technology, Republic of China, 2005.

    [31] S.R.Vaishnav, Z.J.Khan, "Design and Performance of PID and Fuzzy Logic Controller with Smaller Rule Set for Higher Order System" Proceedings of the World Congress on Engineering and Computer Science 2007, WCECS 2007, San Francisco, USA, October 24-26, 2007.

    [32] Anna Vasickaninova, Monika Bakosova and Dalibor Puna, "Fuzzy Logic Control of A Chemical Reactor with Disturbances", 33rd International Conference of SSCHE, May 2006.

Application of fuzzy logic to control acetylene hydrogenation reactor of olefin unit